Nanoscale machines convert light into work - Phys.org

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Researchers created an optical matter machine that operates much like a mechanical machine in which if one gear is turned, a smaller interlocking gear will spin in the opposite direction (a). The optical matter machine (b) uses circularly polarized light to create a nanoparticle array that acts like the larger gear by spinning in the optical field. This makes a probe particle - analogous to the second smaller gear - orbit the nanoparticle array in the opposite direction. Credit: Norbert F. Scherer, University of Chicago

Researchers have developed a tiny new machine that converts laser light into work. These optically powered machines self-assemble and could be used for nanoscale manipulation of tiny cargo for applications such as nanofluidics and particle sorting.

"Our work addresses a long-standing goal in the nanoscience community to create self-assembling nanoscale machines that can perform work in conventional environments such as room temperature liquids," said research team leader Norbert F. Scherer from the University of Chicago.

Scherer and colleagues describe the new nanomachines in Optica. The machines are based on a type of matter known as optical matter in which metal nanoparticles are held together by light rather than the chemical bonds that hold together the atoms that make up typical matter.

"Both the energy for assembling the machine and the power to make it work come from light," said Scherer. "Once the laser light is introduced to a solution containing nanoparticles, the entire process occurs on its own. Although the user does not need to actively control or direct the outcome, this could readily be done to tailor the machines for various applications."

Creating optical matter

In optical matter, a laser light field creates interactions between metal nanoparticles that are much smaller than the wavelength of light. These interactions cause the particles to self-assemble into ordered arrays. This is a similar principle to optical trapping, in which light is used to hold and manipulate particles, biological molecules and cells.

This video shows a simulation of a seven-particle optical matter gear. The spinning and orbiting motion of field (blue) scattered from the nanoparticles (yellow) when circularly polarized light is incident on the nanoparticles can be seen. The rotation of the scattered light (blue) creates the counterclockwise movement of a nanoparticle probe that would enter the optical trap near the gear. The probe particle (not shown here) then orbits as it is relatedly nudged along by the sweep of the motion of the scattered light (blue). The collective rotation of the entire gear is not evident because it occurs on much longer timescales than the femtoseconds timescale motion of the light that is shown here. Credit: Norbert F. Scherer, University of Chicago

In previous work, the researchers discovered that when optical matter is exposed to circularly polarized light, it rotates as a rigid body in the direction opposite the polarization rotation. In other words, when the incident light rotates one way the optical matter array responds by spinning the other. This is a manifestation of "negative torque". The researchers speculated that a machine could be developed based on this new phenomenon.

In the new work, the researchers created an optical matter machine that operates much like a mechanical machine based on interlocking gears. In such machines, when one gear is turned, a smaller interlocking gear will spin in the opposite direction. The optical matter machine uses circularly polarized light from a laser to create a nanoparticle array that acts like the larger gear by spinning in the optical field. This "optical matter gear" converts the circularly polarized light into orbital, or angular, momentum that influences a nearby probe particle to orbit the nanoparticle array (the gear) in the opposite direction.

Determining efficiency

The researchers made two machines based on this design using laser light with a 600-nanometer wavelength and sliver nanoparticles just 150 nanometers in diameter in water. They found that using a gear made of eight nanoparticles created a more efficient machine than a seven-nanoparticle gear, suggesting that the machine's efficiency could be altered by building different gears.

"We believe that what we demonstrated, with further refinement, will be useful in nanofluidics and particle sorting," said John Parker, graduate student and first author. "Our simulations show that a much larger machine made of many more particles should be able to exert more power to the probe, so that is an aspect of refinement that we anticipate pursuing."

The researchers are now experimenting with making machines with many more particles or with particles of different materials. The practicality of the machine could also be improved by creating patterned gears where the nanoparticles are immobile. This would enable the ability to optically address and combine several gears to make a more complex machine.

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More information: John Parker et al, An Optical Matter Machine: Angular Momentum Conversion by Collective Modes in Optically Bound Nanoparticle Arrays, Optica (2020). DOI: 10.1364/OPTICA.396147

Provided by The Optical Society

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